浙江农业学报2024,Vol.36Issue(2) :391-403.DOI:10.3969/j.issn.1004-1524.20221397

基于高频数据的旱地降雨径流污染物输出特征研究

Study on output characteristics of pollutants in rainfall-runoff from upland based on high-frequency data

杨林沛 李金文 沈根祥 朱文俊 陈小华 陈诚 梁利权
浙江农业学报2024,Vol.36Issue(2) :391-403.DOI:10.3969/j.issn.1004-1524.20221397

基于高频数据的旱地降雨径流污染物输出特征研究

Study on output characteristics of pollutants in rainfall-runoff from upland based on high-frequency data

杨林沛 1李金文 2沈根祥 2朱文俊 2陈小华 2陈诚 2梁利权3
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作者信息

  • 1. 东华大学 环境科学与工程学院,上海 201620;上海市环境科学研究院 国家环境保护新型污染物环境健康影响评价重点实验室,上海 200233
  • 2. 上海市环境科学研究院 国家环境保护新型污染物环境健康影响评价重点实验室,上海 200233
  • 3. 华东理工大学 资源与环境工程学院,上海 200237
  • 折叠

摘要

为阐明旱地农田产流特征及面源污染物的排放特征,以上海市崇明岛旱地为研究对象,采用自动取样方法,在自然降雨条件下对旱地径流水文水质进行长期监测.土壤产流能力用径流曲线数(CN)表示,并用高频的电导率(EC)和浊度数据表征可溶性和颗粒态污染物的浓度变化,通过分析浓度 流量(C-Q)关系,从滞后效应角度研究溶解态和颗粒态污染物的输出特征.结果表明,径流系数与降雨量相关性良好,CN与前期土壤含水率(AMC)的相关关系较好.浊度能够反映悬浮泥沙浓度(SSC)、总磷(TP)浓度,EC能够反映可溶性盐的浓度(用全盐量表征).浊度 流量总体上呈现顺时针滞后,冲刷作用明显;EC-流量总体上呈现逆时针滞后,稀释作用明显.TP的输出以冲刷作用为主,总氮(TN)、硝态氮(NO3--N)、氨态氮(NH4+-N)、溶解性总磷(DTP)的输出既有稀释作用也有冲刷作用.TN主要来自土壤溶液,多变的迁移路径是溶解态物质输出大多呈现逆时针滞后的原因.TP主要来自土壤表面,较短的迁移路径是颗粒态污染物输出大多呈现出顺时针滞后模式的原因.本研究获得的溶解态和颗粒态污染物的输出过程和特征可为面源污染防控、水土保持提供科学依据.

Abstract

In order to clarify output characteristics of different forms of pollutant discharge from upland under rainfall event,the long-term monitoring of runoff and water quality in farmland under natural rainfall was carried out by means of automatic sampling on Chongming Island in Shanghai,China.High-resolution electrical conductivity(EC)and turbidity measurements were used to indicate the concentrations of dissolved and particulate nutrients respective-ly.The runoff curve number(CN)was used to represent the runoff production capacity.The output characteristics of nutrients from upland was studied by the hysteresis loop analysis,which was indicated by concentration-discharge(C-Q)relationship.The results showed that there was a good correlation between runoff coefficient and rainfall,and the CN was well related to soil moisture content(AMC).EC and turbidity could be used as surrogates of soluble salt content(represented by the total salt content),and suspended sediment concentration(SSC)and total phosphorus(TP)concentration,respectively.Turbidity-discharge generally showed clockwise hysteresis and obvious flush effect.Generally,the EC-discharge showed anticlockwise hysteresis,and dilution effect.The output of TP was main-ly due to flush effect.The output characteristics of total nitrogen(TN),nitrate nitrogen(NO-3-N),ammonium ni-trogen(NH+4-N)and soluble total phosphorus(DTP)were highly variable,which had both dilution and flush effects.It was included that the dissolved form of nutrients such as N-related pollutants was probably transported through both soil surface and cultivated layer.Nevertheless,as particulate pollutants,TP mainly transported on soil surface,and that was the reason why the output of particulate pollutants mostly showed a clockwise hysteresis pat-tern.The output process and characteristics of dissolved and particulate pollutants provided scientific basis for the control of non-point source pollution and soil and water conservation.

关键词

原位监测/降雨产流/高分辨率/面源污染

Key words

in-situ monitoring/rainfall-runoff/high-resolution/non-point source pollution

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基金项目

上海市生态环境局科研项目(沪环科[2020]第5号)

出版年

2024
浙江农业学报
浙江省农业科学院 浙江省农学会

浙江农业学报

CSTPCDCSCD北大核心
影响因子:0.765
ISSN:1004-1524
参考文献量42
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