首页|Fluorescent graphitic carbon nitride with photocatalytic oxidase-like activity for anti-counterfeiting application
Fluorescent graphitic carbon nitride with photocatalytic oxidase-like activity for anti-counterfeiting application
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NSTL
Elsevier
Herein bulk phenyl- and carbon-modified graphitic carbon nitride (PCCN) powders with tunable fluorescent emission from green-color to yellow-color were prepared by copolymerization of 2,4-diamino-6-phe nyl-1,3,5-triazine and 2,2,6-triaminopyrimidine. The corresponding nanosheets with blue-color to green-color fluorescence were obtained by the oxidation of their bulk powders in sulfuric or nitric acid and then ultrasonic exfoliation. The typical PCCN0.6 nanosheets not only displayed strong green-color fluorescence but also exhibited photocatalytic oxidase-like activity, which can catalyze the oxidation of substrates 3,3',5,5'-tetramethylbenzidine and Amplex UltraRed by O-2 to produce blue-color colorimetric product and pink-color fluorescent product, respectively. By taking advantage of green-color fluorescence and photocatalytic activity of PCCN0.6 nanosheets, a prototype for high-level anti-counterfeiting application was demonstrated by using the mixture of PCCN0.6 nanosheets and Amplex UltraRed as the fluorescent ink. (C) 2021 Elsevier B.V. All rights reserved.
NSTL
Elsevier
